As she nears 40, and with six young children in tow, she tells us she's ready to slow things down.
"Yes, I'm going to take more of a back seat," Angelina confirmed to us last week.
"I've had a wonderful career and I'm very happy I've had the opportunity to tell stories and work for as long as I have."
She adds: "I'm sure there will be a few more films but I'm happy to be selective.
"I want to focus more on writing and directing and, above all, I would like to focus more on my work with the UN (United Nations) and PSBI (Pearl S Buck International child charity)."
Sadly, her new role as Maleficent, the evil character who put a spell on young Sleeping Beauty, may be one of her last.
The twice-divorced star – who is rumoured to be marrying Brad Pitt, the dad of their six children, later this year – also gave us an insight into her "normal as can be" family life at the press conference for her new movie, Maleficent, in London.
"I usually make up stories for my kids. I like to tell them stories every night and I make up any kind of crazy thing!" she told us.
"But I don't like the idea that there are always happy endings, or that there is just good and evil, or things are perfect. I like a moral tale and I think that's what I try and teach my kids."
Naturally, they are particularly taken with Mr and Mrs Smith – the film in which Brangelina play married spies tasked to kill each other, and in which their romance first blossomed.
"The older kids recently watched Mr and Mrs Smith and they thought it was the funniest thing in the world. Watching your parents fight as spies is some strange child fantasy!" she laughed.
Would they like to see their mum and dad do a sequel to the movie?
"Of Mr and Mrs Smith? I feel like I've lived out the rest of that one!" she jokes.
Read the whole interview in this week's Reveal magazine – out now!
Reveal is now on Google Plus! Join us here for the latest pictures, fashion and celebrity news!
Got an iPad or iPhone? Reveal Mag is specially designed to fit!