The 25-year-old 'Skyfall' singer took to Twitter to praise the hip-hop artist after he performed 'Bound 2', taken from his critically acclaimed album, Yeezus.
Kanye flew into London to record a special taping for the show, which aired last night on BBC Two and the rapper performed a stripped-back version of the song alongside R&B legend Charlie Wilson.
Watching from the comfort of her own sofa, mum-of-one Adele tweeted: "God I love Kanye so much. Later with Jools is incredible tonight!"
Adele, who was last seen enjoying Lady Gaga's concert at the iTunes Festival earlier this month, doesn't tweet too often, so we reckon she must have been really impressed with Kanye's performance! We'd love to see the two music stars collaborate in the near future!
Kanye performed his track alongside the likes of Sting and Kings of Leon on the 30 minute show. The rapper can be seen performing more tracks in an extended version of the show to air on Friday (20 September).
Watch Kanye's performance of 'Bound 2' below: